图书简介
The Proceedings of the 24th International Solvay Conference on Chemistry comprise contributed short personal statements and transcripts of in-depth discussions on "Catalysis in Chemistry and Biology" from a by-invitation-only select group of 48 eminent scientists, including four Nobel Laureates, from all parts of the world. The theme of the conference was presented in six sessions, along which the Proceedings are organized. The first session on "Homogeneous Catalysis, " chaired by Professor Robert Grubbs, is devoted to basic research on catalysis in homogeneous solutions and applications thereof. "Heterogeneous Catalysis and Characterization of Catalyst Surfaces, " chaired by Professor Gerhard Ertl, includes extensive references to industrial applications of catalysis on solid supports, and discussions on the experimental techniques used in this field. "Catalysis by Microporous Materials, " chaired by Professor Mark E. Davis, is devoted to a detailed characterization of this particular class of solid support catalysts, with special emphasis on model analysis of the processes catalyzed by these materials. "Catalysis under Extreme Conditions: Studies at High Pressure and High Temperatures — Relations with Processes in Nature, " chaired by Professor Henk N W Lekkerkerker, broadens the scope of the two preceding sessions with exciting illustrations. The sessions on "Catalysis by Protein Enzymes, " chaired by Prof. JoAnne Stubbe, and "Catalysis by Ribozymes in Molecular Machines, " chaired by Prof. David Lilley, present at the same time an exciting extension of and a contrast to the initial four sessions. The combination of the six sessions provides an impressive overview, giving innovative insights into relationships between catalysis in chemical processes and in biological systems, and a unique outlook to anticipated developments in the coming years and the more distant future.
Key Features:
○ The authors are my collaborators and leaders in the field
○ The chapter presentations — with glossaries, definitions of abbreviations, generous color figures and tables — is designed to be more straightforward and less complicated than many of the papers the data is derived from
○ Furthermore, after the presentation of data, summaries reiterate the relevant points and take-home messages
Opening Address (M Henneaux); Preface (K Wüthrich); Session 1: Homogeneous Catalysis: Homogeneous Catalysis: Organometallic Catalysis and Organocatalysis (R H Grubbs); Copper-Catalyzed Hydrofunctionalization Reactions (S L Buchwald); Controlling Selectivity and Reactivity in Catalytic C–H Functionalization Reactions (M Sanford); Designing New Homogeneous Transition Metal Catalysts for Aerobic Oxidations (K I Goldberg); Organocatalysis — From Laboratory Scale to Industrial Processes (K A Jørgensen); Homogeneous Catalysis in the Future (E M Carreira); Exploring Chemical Space in Homogeneous Catalysis (B L Feringa); Ligands with Intrinsic Donor Flexibility for Redox Catalysis (M Albrecht, M Navarro, C Segarra); Development of New Catalysts Toward Utilization of Renewable Resources (R Nakano, S Kusumoto, K Nozaki); Challenges for Organocatalysis (B List); Discussions of Session 1; Session 2: Heterogeneous Catalysis and Characterization of Catalyst Surfaces: Heterogeneous Catalysis: Where are We? (G Ertl); Integration of the Three Fields of Catalysis: Heterogeneous, Homogeneous, and Enzyme (G A Somorjai, R Ye, T J Hurlburt, K Sabyrov); Towards a Theory of Heterogeneous Catalysis (J K Nørskov); Structure-Reactivity Relations Through Charge Control at the Atomic Level in Heterogeneous Catalysis (H-J Freund); Computational Catalysis: Rigor and Relevance (J Sauer); Heterogeneous Catalysis Using Supported Gold and Gold Palladium Nanostructures: Understanding the Nature of the Active Species (G J Hutchings); Heterogeneous Catalysis, Understanding the Micro to Build the Macro (A Corma); Heterogenous Catalysis and Characterization of Catalyst Surfaces (J M Thomas); Discussions of Session 2; Session 3: Catalysis by Microporous Materials: Catalysis by Crystalline, Microporous Materials (M E Davis); Can We Predict the Reactivity of the Zeolite Catalyst? (R A van Santen, C Liu, E A Pidko, E J M Hensen); Consequences of Confinement for Catalysis within Voids of Molecular Dimensions (E Iglesia); Advanced Zeolites with Heteroatom Site Distribution in the Framework Controlled (T Tatsumi); Evolution Trends in Zeolite-Based Catalysts (G Bellussi, R Millini); Molecular Sieve Zeotypes — Targeting Structure Types Through Synthesis Design (J L Casci, R Garcia, A Turrina, P A Wright, P A Cox); Catalysis by Microporous Metal Organic Frameworks (C W Jones, L Darunte, K Eum, S Pang, G Zhu, S A Didas, S Nair); Discussions of Session 3; Session 4: Catalysis Under Extreme Conditions: Studies at High Pressure and High Temperatures — Relations with Processes in Nature: Catalysis Under Extreme Conditions: Studies at High Pressure and High Temperatures & Their Relations with Processes in Nature (H N W Lekkerkerker); Electron Microscopy in Heterogeneous Catalysis (S Helveg); Operando Spectroscopy of a Catalytic Solid: Towards a Molecular Movie (B M Weckhuysen); Novel Concepts in C1 Chemistry (X Bao); Electrochemistry for the Production of Fuels, Chemicals and Materials (M T M Koper); Electrocatalysis at Deep-Sea Hydrothemal Vents (R Nakamura); Controlled Functionalisation and Understanding of Surfaces Towards Single Site Catalysts and Beyond (C Copé ret); Discussions of Session 4; Session 5: Catalysis by Protein Enzymes: Biological Catalysis: Understanding Rate Accelerations in Enzymatic Reactions (J Stubbe); Top-Down and Bottom-Up Approaches For Elucidating the Origins of Enzyme Efficiency (D Hilvert); Electric Fields and Enzyme Catalysis (S G Boxer, S D Fried, S H Schneider, Y Wu); Water Mapping in Enzymatic Catalysis by Thz Spectroscopy (Thz Calorimetry) (M Havenith); Theory of Single Molecule Experiments of F1-ATPase: Predictions, Tests and Comparison with Experiments (S Volkán-Kacsó , RA Marcus); Interplay of High-Level Spectroscopy and Quantum Chemistry: A Powerful Tool to Unravel Enzymatic Reaction Mechanisms (F Neese); Protein Dynamics in Enzymatic Catalysis (B Dyer, M J Reddish, R Callender); How Close are We to Explaining Enzyme Catalysis? (J P Klinman, S Hu, A Offenbacher); Discussions of Session 5; Session 6: Catalysis by Ribozymes in Molecular Machines: Mechanistic Origins of RNA Catalysis (D M J Lilley); Catalytic Strategies of Nucleolytic Ribozymes (D M York); Key Catalytic Strategies of Ribozymes (P C Bevilacqua, J L Bingaman, E A Frankel, K J Messina, D D Seith); Prospects for Ribozyme Discovery and Analysis (R R Breaker); The Ribosome as a Catalyst of GTP Hydrolysis by Translational GTPases (M V Rodnina); Lessons from Catalysis by RNA Enzymes (D Herschlag, R Sengupta); Discussions of Session 6; Index
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