图书简介
This book introduces the physical, chemical, and biological principles underlying photosynthesis. It addresses the underlying physics of light harvesting and key spectroscopic methods, including data analysis, andcovers theassembly of the natural system, its energy transfer properties, and regulatory mechanisms.
Introduction. Part 1. Building the light-harvesting apparatus: Pigments. Chlorophylls: Biosynthesis and general properties. Chlorophylls in a protein environment: How to calculate their spectral and redox properties (From MO to DFT . Carotenoids; Biology, functions, electronic states, Part 2. Building the light-harvesting apparatus: Proteins. Light-harvesting in higher plants and green algae. Light-harvesting in cyanobacteria (phycobilisomes, etc.). The purple bacterial photosynthetic apparatus. Green sulfur bacteria (FMO and chlorosomes): Chlorosomes, structure, self-organized BChl c aggregates, EET properties, baseplate, FMO, EET to the RC. Light harvesting complexes in Chl c - containing algae. Reaction center: The bacterial RC. Part 3. Light-harvesting systems in action: Energy transfer and electron transport. Introduction, open questions, etc. Exciton concept. Exciton transfer dynamics 1: Redfield vs. Forster. Exciton transfer dynamics 2 - new theory HIEM etc. Quantum aspects of energy transfer. Electron transfer. Modulation of the redox potentials. Part 4. Light-harvesting systems in action: Spectroscopy. Basic spectroscopy for light-harvesting. Advanced spectroscopy: Ultrafast and 2D. Experimental evidence for quantum coherence in photosynthetic light harvesting. Data Analysis: Global and target analysis, systems biology. Part 5. Assembling the natural system. Assembly of the thylakoid membrane. Energy transfer in the membranes of plants. Energy transfer in the bacterial membrane LH2, LH1, RC, the chromatophore, pufX, curvature, dimeric RCs vs randomly positioned RCs. Non-photochemical quenching. Part 6. Artificial Photosynthesis. A Study of light harvesting, photoregulation and photoprotection in selected artificial photosynthetic systems. Light-harvesting in organic/dye-sensitized solar cells. Part 7. Photosynthesis in the Sun. Photosynthesis in leaves: Chlorophyll fluorescence and other biophysical techniques. Harvesting sunlight with cyanobacteria and algae for sustainable production in a bio-based economy. Environmental Physics of Photosynthesis. Photosynthesis and artificial photosynthesis in the Sun.
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